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I checked the throttle body synchronization on my '85 LTD. It did not need an adjustment. The engine vacuum is what it is, and cannot be changed. The idea is to get the right side and left side as close to the same as possible. On the LTD (fuel injected) all you can do is synchronize the right side to the left. There is NO adjustment possible between the front and rear, as they use the same throttle shaft. If you synchronize the right and left rear, and get them both the same, then check the right and left front, and find they are off, then there is either an issue with the front cylinders themselves, or something in the throttle linkage is bent. If you then try to synchronize the front, and make any adjustments, the rear will be off.
I keep hearing how there is one carb that cannot be changed, and you have to synchronize the other 3 to that one. I have no clue what that means. Is the carb setup completely different from the FI setup? With the FI, you CANNOT synchronize the front and rear carbs relative to each other. I have one of the old Motion Pro mercury synchronizers, the really tall one that must be kept upright so the mercury doesn't run out, and it worked fine. I didn't even check the front 2 throttle bodies, I checked the right rear and left rear. It wouldn't do any good to check the front anyway, as there is nothing you can do about it if they are off, without messing up the rear. The engine runs fine, so I see no reason to worry about it. I guess I'm going to have to take a closer look at how the carb setup is designed.